CCL:G: mail from Joshi



Perhaps things have changed, and I've forgotten that, but I know that STO-NG* basis sets put d orbitals on the Na-Cl row of the periodic table, and I thought the same was true for 3-21G*.. Am I incorrect?

Also,  why not try PM6/MOPAC2007 for this for a starting pass at the geometry, along with AIGOUT which prepares a GXY input geometry Z-Matrix?

Cheers!

John McKelvey

On Mon, Nov 3, 2008 at 8:17 AM, Marcel Swart marcel.swart|*|icrea.es <owner-chemistry%x%ccl.net> wrote:
Note also the following paper, for hydrocarbons it gives good and fast results (seconds on regular PC):

http://dx.doi.org/10.1021/ct8003222

Thermochemistry of Hydrocarbons. Back to Extended Hückel Theory

On Nov 3, 2008, at 10:41 AM, Kalju Kahn kalju]=[chem.ucsb.edu wrote:


Sent to CCL by: "Kalju Kahn" [kalju:+:chem.ucsb.edu]
Joshi,

Are you sure that you need B3LYP/3-21G* geometry for this structure? 
Seems like molecular mechanics with MM3 might be better suited for
optimizing a large hydrocarbon.

If you need DFT geometry for some reason, try to freeze all dihedrals and
optimize bond distances and angles first.  Small deviations of torsional
angles around single bonds is more acceptable than an unusually stretched
bond for calculation of some molecular properties.

Kalju

Dear CCLers; Hi

I am optimizing a molecule having 387 atoms (only C and H atoms) which
includes neatly 16 methyl groups as substitutions in G03w, and the method
is b3lyp/3-21g*. During the optimization the Maximum Force
and RMS Forces are sometimes converging, Maximum
Displacement and RMS     Displacements are not converging and the
molecules energy is oscillating. I am using following keywords in route
section as

%mem=1500mb
%nproc=4
#p opt=(gdiis,maxcycle=200) b3lyp/3-21g* scf=maxcycle=500

Please give me suggestion

Thanks in advance

Joshi



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Department of Chemistry and Biochemistry
UC Santa Barbara, CA 93106



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