CCL:G: Finding the transition state



Hi Juan, Have you tried a QST3? In addition to the reactants and products, this will allow you to use input an initial guess for the transition state.

Additionally, you could get an estimate of the reaction path using opt=path from the optimized reactant. The highest energy point along the path can be used as an estimate for the transition state of the QST3 calc, while the step down the gradient on the reactant side may be used as the reactant guess in the QST3, and so on for the product.

Whichever method you use, I would run an IRC once you are finished to ensure the transition state you've calculated is the for the reaction you intended.

Good luck,

Amy



From: Juan Manuel mayerzmytm#%#gmail.com <owner-chemistry-#-ccl.net>
To: "Austin, Amy J " <amy_jean_austin-#-yahoo.com>
Sent: Monday, July 15, 2013 12:13 PM
Subject: CCL:G: Finding the transition state

Hello Ailar,

I have not a lot of experience working with theoretical methods, but something that worked to me in order to find transition structure is use the berny method (only TS initial guess needed) with the keyword NoEigenTest, otherwise I found this process very dificult

opt=(ts,noeigentest).......

best

Juan Manuel Arce


2013/7/12 Ailar Badri ailar121242363:-:yahoo.co.uk <owner-chemistry]=[ccl.net>

Sent to CCL by: "Ailar  Badri" [ailar121242363-.-yahoo.co.uk]
Dear CCLers,

I'm looking for transition state structure using qst2 command, but I have not been succeed so far. I tried many kinds of reactant/product structures to find the transition state. However, my calculations always terminate with the following error almost immediately after submitting the job:

Old curvilinear step not converged, using linear step:
 SCX= 2.80D+01 DXMaxT= 5.30-317 SCLim= 0.00D+00 Fact= 0.00D+00
 RedCar/ORedCr failed for GTrans.
 Error termination via Lnk1e in /afs/ics.muni.cz/software/g09-D01/em64t.sse4.2/g09/l101.exe at Fri Jul 12 15:31:42 2013.

I would be grateful if someone can help me. I am using Gaussian 09 rev. D01.

Regards,
Ailar Badri



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