CCL:G: Gaussian error in Frequency Calculation



 Sent to CCL by: Igors Mihailovs [igorsm[-]cfi.lu.lv]
 Hello Dr. Kraemer,
 
Not to help probably, but I have once encountered this in a calculation which does not utilize any dispersion correction at all. It was an LC-BLYP calculation using Linda, which somehow failed to even start (all force constants were NaN at the first iteration) but did not notice this and continued for 199 steps at which it signalled "Number of steps exceeded" (with all four optimization parameters "converged"). Also, at the end of the estimation of the Hessian (even at the very beginning) the following message is printed:
 RFO could not converge Lambda in  999 iterations.
 The route section was:
 #T LC-BLYP/6-311G(d,p) Opt(Tight) Integral(Grid=UltraFineGrid) SCRF(So
  lvent=Chloroform) Guess=Mix
 
Back then I then resorted to think this was a technical issue. The excerpt of the output is below:
 Electronic spatial extent (au): 
 <R**2>=          
 9159.2106
  Charge=             
 0.0000 electrons
  Dipole moment (field-independent basis, Debye):
 
    X=              4.6583    Y=             -2.0724 Z=              0.0000  Tot=              5.0985
   Exact polarizability: 530.016 -25.136 261.274  
 0.000   0.000 105.036
  Approx polarizability: 310.731 -12.857 234.854  
 0.000   0.000 111.144
  Rotating derivatives to standard orientation.
  Full mass-weighted force constant matrix:
  Low frequencies ---      
 NaN       NaN      
 NaN       NaN
 NaN       NaN
  Low frequencies ---      
 NaN       NaN      
 NaN
  Diagonal vibrational polarizability:
              
 NaN            
 NaN             NaN
  Harmonic frequencies (cm**-1), IR intensities (KM/Mole), Raman scattering
  activities (A**4/AMU), depolarization ratios for plane and unpolarized
  incident light, reduced masses (AMU), force constants (mDyne/A),
  and normal coordinates:
                      
 1
 2                     
 3
                     
 A'                    
 A' A'
  Frequencies --         NaN
 NaN                   
 NaN
  Red. masses --         NaN
 NaN                   
 NaN
  Frc consts  --         NaN
 NaN                   
 NaN
  IR Inten   
 --         NaN
 NaN                   
 NaN
   Atom  AN     
 X      Y     
 Z        X     
 Y      Z X     
 Y      Z
      1   6     
 NaN    NaN    NaN     
 NaN    NaN    NaN NaN   
 NaN    NaN
      2   6     
 NaN    NaN    NaN     
 NaN    NaN    NaN NaN   
 NaN    NaN
      3   6     
 NaN    NaN    NaN     
 NaN    NaN    NaN NaN   
 NaN    NaN
      4   6     
 NaN    NaN    NaN     
 NaN    NaN    NaN NaN   
 NaN    NaN
      5   6     
 NaN    NaN    NaN     
 NaN    NaN    NaN NaN   
 NaN    NaN
      6   6     
 NaN    NaN    NaN     
 NaN    NaN    NaN NaN   
 NaN    NaN
 Hope this at least eliminates some wrong paths of possible resolutions.
 Regards,
 IM
 On 11/2/20 11:11 PM, Tobias Kraemer tobias.kraemer .. mu.ie wrote:
 
 Sent to CCL by: "Tobias  Kraemer" [tobias.kraemer[-]mu.ie]
 Hello all,
 I hope everyone is well. I haven't posted here for a long time, but I have
 encountered some strange
 behaviour in a Gaussian frequency calculation that I have not seen before. There
 seems to be little to
 no information out there on this problem, so I was hoping to get some input from
 the list.
 Essentially, we are running a geometry optimisation with subsequent frequency
 job (same input)
 at the B3LYP/6-311+G(d) level of theory and including the GD3BJ dispersion
 correction. The molecule
 is a small molecules containing potassium. The optimisation furnishes a
 perfectly fine structure, but
 the calculation then error terminates with the following message
 Maximum of*** iterations exceeded in RedStp.
 All entries in this section contain NaN entries, e.g.
 Frequencies --         NaN                    NaN                    NaN
   Red. masses --         NaN                    NaN                    NaN
   Frc consts  --         NaN                    NaN                    NaN
   IR Inten    --         NaN                    NaN                    NaN
    Atom  AN      X      Y      Z        X      Y      Z        X      Y      Z
       1  19      NaN    NaN    NaN      NaN    NaN    NaN      NaN    NaN    NaN
       2   6      NaN    NaN    NaN      NaN    NaN    NaN      NaN    NaN    NaN
       3   1      NaN    NaN    NaN      NaN    NaN    NaN      NaN    NaN    NaN
       4   1      NaN    NaN    NaN      NaN    NaN    NaN      NaN    NaN    NaN
       5   6      NaN    NaN    NaN      NaN    NaN    NaN      NaN    NaN    NaN
       6   6      NaN    NaN    NaN      NaN    NaN    NaN      NaN    NaN    NaN
 Obviously something has gone awfully wrong in the frequencies. The problem can
 be reproduced by
 running the frequency job on the optimised geometry alone (here we used a
 smaller basis set).
 Interestingly the calculation finishes normally in this case, but shows only NaN
 entries everywhere in
 the output.
 I have seen some indication that this may be related to the D3 correction, but I
 would like to hear your
 opinion on this. We are running G09 E.01.
 your help would be much appreciated. thanks in advance.
 Kind regards,
 Tobias>